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The sizes and shapes of ice crystals influence the radiative properties of clouds, as well as precipitation initiation and aerosol scavenging. However, ice crystal growth mechanisms remain only partially characterized. We present the growth processes of two complex ice crystal habits observed in Arctic mixed-phase clouds during the Ny-Ålesund AeroSol Cloud ExperimeNT campaign. First, are capped-columns with multiple columns growing out of the plates' corners that we define as columns on capped-columns. These ice crystals originated from cycling through the columnar and plate temperature growth regimes, during their vertical transport by in-cloud circulation. Second, is aged rime on the surface of ice crystals having grown into faceted columns or plates depending on the environmental conditions. Despite their complexity, the shapes of these ice crystals allow to infer their growth history and provide information about the in-cloud conditions. Additionally, these ice crystals exhibit complex shapes and could enhance aggregation and secondary ice production. Geophysical Research Letters, 50 (1) ISSN:1944-8007 ISSN:0094-8276

The ISONET project has been striving to improve greatly our understanding of European climate systems providing independent quantitative data for model verification and policy making. A network of 24 sites provides dendrochronological coverage from Iberia to Fennoscandia, Caledonia and the Tyrol. The stable isotope (C, H, O) ratios of these annually resolved time series shall be analysed within this project, to reconstruct past climate regimes (temperature, relative humidity and precipitation characteristics) for the last 400 years. Climate variability shall be addressed on three timescales; decade-century (source water/air mass dominance); inter-annual (quantifying baseline variability, extreme events and recent trends); and intra-annual (high resolution exploration of seasonality signals within tree-rings). ISONET goes far beyond existing tree-ring analyses in its spatial based investigation and interpretation (see also https://cordis.europa.eu/project/id/EVK2-CT-2002-00147). 24 European annually resolved stable isotope chronologies have been constructed from tree ring cellulose for the last 400 years (1600CE – 2003CE) for carbon and oxygen and for the last 100 years for hydrogen. Data was produced within the ISONET project (400 Years of Annual Reconstructions of European Climate Variability Using a Highly Resolved Isotopic Network,) to initiate an extensive spatiotemporal tree-ring stable isotope network across Europe funded as part of the fifth EC Framework Programme “Energy, Environment and Sustainable Development”. This data set comprises the ISONET δ13C records. Wood increment cores of 15 or more Pinus sylvestris, Quercus robur/petraea or Cedrus atlantica tree individuals were taken. Dendro-dated tree-ring material of 4-5 individuals per site was dissected and pooled year by year. After cellulose extraction and homogenization, 18O/16O-ratios of annually resolved samples were determined by Isotope Ratio Mass Spectrometry (IRMS). Time series of 13C/12C are given as d-values versus PDB. Details can be found in the downloadable “data description” file.

The ISONET project has been striving to improve greatly our understanding of European climate systems providing independent quantitative data for model verification and policy making. A network of 24 sites provides dendrochronological coverage from Iberia to Fennoscandia, Caledonia and the Tyrol. The stable isotope (C, H, O) ratios of these annually resolved time series shall be analysed within this project, to reconstruct past climate regimes (temperature, relative humidity and precipitation characteristics) for the last 400 years. Climate variability shall be addressed on three timescales; decade-century (source water/air mass dominance); inter-annual (quantifying baseline variability, extreme events and recent trends); and intra-annual (high resolution exploration of seasonality signals within tree-rings). ISONET goes far beyond existing tree-ring analyses in its spatial based investigation and interpretation (see also https://cordis.europa.eu/project/id/EVK2-CT-2002-00147). 24 European annually resolved stable isotope chronologies have been constructed from tree ring cellulose for the last 400 years (1600CE – 2003CE) for carbon and oxygen and for the last 100 years for hydrogen. Data was produced within the ISONET project (400 Years of Annual Reconstructions of European Climate Variability Using a Highly Resolved Isotopic Network,) to initiate an extensive spatiotemporal tree-ring stable isotope network across Europe funded as part of the fifth EC Framework Programme “Energy, Environment and Sustainable Development”. This data set comprises the ISONET δ18O records. Wood increment cores of 15 or more Pinus sylvestris, Quercus robur/petraea or Cedrus atlantica tree individuals were taken. Dendro-dated tree-ring material of 4-5 individuals per site was dissected and pooled year by year. After cellulose extraction and homogenization, 18O/16O-ratios of annually resolved samples were determined by Isotope Ratio Mass Spectrometry (IRMS). Time series of 18O/16O are given as d-values versus SMOW. Details can be found in the downloadable “data description” file.

The Arctic is very susceptible to climate change and thus is warming much faster than the rest of the world. Clouds influence terrestrial and solar radiative fluxes and thereby impact the amplified Arctic warming. The partitioning of thermodynamic phases (i.e., ice crystals and water droplets) within mixed-phase clouds (MPCs) especially influences their radiative properties. However, the processes responsible for ice crystal formation remain only partially characterized. In particular, so-called secondary ice production (SIP) processes, which create supplementary ice crystals from primary ice crystals and the environmental conditions that they occur in, are poorly understood. The microphysical properties of Arctic MPCs were measured during the Ny-Ålesund AeroSol Cloud ExperimENT (NASCENT) campaign to obtain a better understanding of the atmospheric conditions favorable for the occurrence of SIP processes. To this aim, the in situ cloud microphysical properties retrieved by a holographic cloud imager mounted on a tethered balloon system were complemented by ground-based remote sensing and ice-nucleating particle measurements. During the 6 d investigated in this study, SIP occurred during about 40 % of the in-cloud measurements, and high SIP events with number concentrations larger than 10 L−1 of small pristine ice crystals occurred in 4 % of the in-cloud measurements. This demonstrates the role of SIP for Arctic MPCs. The highest concentrations of small pristine ice crystals were produced at temperatures between −5 and −3 ∘C and were related to the occurrence of supercooled large droplets freezing upon collision with ice crystals. This suggests that a large fraction of ice crystals in Arctic MPCs are produced via the droplet-shattering mechanism. From evaluating the ice crystal images, we could identify ice–ice collision as a second SIP mechanism that dominated when fragile ice crystals were observed. Moreover, SIP occurred over a large temperature range and was observed in up to 80 % of the measurements down to −24 ∘C due to the occurrence of ice–ice collisions. This emphasizes the importance of SIP at temperatures below −8 ∘C, which are currently not accounted for in most numerical weather models. Although ice-nucleating particles may be necessary for the initial freezing of water droplets, the ice crystal number concentration is frequently determined by secondary production mechanisms. Atmospheric Chemistry and Physics, 22 (23) ISSN:1680-7375 ISSN:1680-7367

Abstract. We present an age model for the 651 m deep Skytrain Ice Rise ice core. The top 2000 years have previously been dated using age markers interpolated through annual layer counting. Below this, we align the Skytrain core to the AICC2012 age model using tie points in the ice and air phase, and apply the Paleochrono program to obtain the best fit to the tie points and glaciological constraints. In the gas phase, ties are made using methane and, in critical sections, δ18Oair; in the ice phase ties are through 10Be across the Laschamps Event, and through ice chemistry related to long-range dust transport and deposition. This strategy provides a good outcome to about 108 ka (~605 m). Beyond that there are signs of flow disturbance, with a section of ice probably repeated. Nonetheless values of CH4 and δ18Oair confirm that part of the last interglacial (LIG), from about 117–126 ka (617–628 m), is present and in chronological order. Below this there are clear signs of stratigraphic disturbance, with rapid oscillation of values in both the ice and gas phase at the base of the LIG section. Based on methane values, the warmest part of the LIG and the coldest part of the penultimate glacial are missing from our record. Ice below 631 m appears to be of age >150 ka.

Solar radiation received at the Earth's surface (Rs) is comprised of two components, the direct radiation (Rd) and the diffuse radiation (Rf). Rd, the direct beam from the sun, is essential for concentrated solar power generation. Rf, scattered by atmospheric molecules, aerosols, or cloud droplets, has a fertilization effect on plant photosynthesis. But how Rd and Rf change diurnally is largely unknown owing to the lack of long-term measurements. Taking advantage of 22 years of homogeneous hourly surface observations over China, this study documents the climatological means and evolutions in the diurnal cycles of Rd and Rf since 1993, with an emphasis on their implications for solar power and agricultural production. Over the solar energy resource region, we observe a loss of Rd which is relatively large near sunrise and sunset at low solar elevation angles when the sunrays pass through the atmosphere on a longer pathway. However, the concentrated Rd energy covering an average 10-hr period around noon during a day is relatively unaffected. Over the agricultural crop resource region, the large amounts of clouds and aerosols scattering more of the incoming light result in Rf taking the main proportion of Rs during the whole day. Rf resources and their fertilization effect in the main crop region of China further enhances since 1993 over almost all hours of the day. Key Points: - The loss of direct radiation over China since 1993 is relatively large at sunrise and sunset with little effect on solar power generation - The diffuse component dominates solar radiation normally near sunrise and sunset, but for the whole day over the main sown area of China - The diffuse fraction is further enhanced in the main sown area of China over almost all hours of the day since 1993

AbstractOver a five-month time window between March and July 2020, scientists deployed two small uncrewed aircraft systems (sUAS) to the central Arctic Ocean as part of legs three and four of the MOSAiC expedition. These sUAS were flown to measure the thermodynamic and kinematic state of the lower atmosphere, including collecting information on temperature, pressure, humidity and winds between the surface and 1 km, as well as to document ice properties, including albedo, melt pond fraction, and open water amounts. The atmospheric state flights were primarily conducted by the DataHawk2 sUAS, which was operated primarily in a profiling manner, while the surface property flights were conducted using the HELiX sUAS, which flew grid patterns, profiles, and hover flights. In total, over 120 flights were conducted and over 48 flight hours of data were collected, sampling conditions that included temperatures as low as −35 °C and as warm as 15 °C, spanning the summer melt season.

International audience; Accurate assessment of anthropogenic carbon dioxide (CO2) emissions and their redistribution among the atmosphere, ocean, and terrestrial biosphere in a changing climate is critical to better understand the global carbon cycle, support the development of climate policies, and project future climate change. Here we describe and synthesize datasets and methodology to quantify the five major components of the global carbon budget and their uncertainties. Fossil CO2 emissions (EFOS) are based on energy statistics and cement production data, while emissions from land-use change (ELUC), mainly deforestation, are based on land use and land-use change data and bookkeeping models. Atmospheric CO2 concentration is measured directly, and its growth rate (GATM) is computed from the annual changes in concentration. The ocean CO2 sink (SOCEAN) is estimated with global ocean biogeochemistry models and observation-based data products. The terrestrial CO2 sink (SLAND) is estimated with dynamic global vegetation models. The resulting carbon budget imbalance (BIM), the difference between the estimated total emissions and the estimated changes in the atmosphere, ocean, and terrestrial biosphere, is a measure of imperfect data and understanding of the contemporary carbon cycle. All uncertainties are reported as ±1σ. For the first time, an approach is shown to reconcile the difference in our ELUC estimate with the one from national greenhouse gas inventories, supporting the assessment of collective countries' climate progress. For the year 2020, EFOS declined by 5.4 % relative to 2019, with fossil emissions at 9.5 ± 0.5 GtC yr-1 (9.3 ± 0.5 GtC yr-1 when the cement carbonation sink is included), and ELUC was 0.9 ± 0.7 GtC yr-1, for a total anthropogenic CO2 emission of 10.2 ± 0.8 GtC yr-1 (37.4 ± 2.9 GtCO2). Also, for 2020, GATM was 5.0 ± 0.2 GtC yr-1 (2.4 ± 0.1 ppm yr-1), SOCEAN was 3.0 ± 0.4 GtC yr-1, and SLAND was 2.9 ± 1 GtC yr-1, with a BIM of -0.8 GtC yr-1. The global atmospheric CO2 concentration averaged over 2020 reached 412.45 ± 0.1 ppm. Preliminary data for 2021 suggest a rebound in EFOS relative to 2020 of +4.8 % (4.2 % to 5.4 %) globally. Overall, the mean and trend in the components of the global carbon budget are consistently estimated over the period 1959-2020, but discrepancies of up to 1 GtC yr-1 persist for the representation of annual to semi-decadal variability in CO2 fluxes. Comparison of estimates from multiple approaches and observations shows (1) a persistent large uncertainty in the estimate of land-use changes emissions, (2) a low agreement between the different methods on the magnitude of the land CO2 flux in the northern extra-tropics, and (3) a discrepancy between the different methods on the strength of the ocean sink over the last decade. This living data update documents changes in the methods and datasets used in this new global carbon budget and the progress in understanding of the global carbon cycle compared with previous publications of this dataset (Friedlingstein et al., 2020, 2019; Le Quéré et al., 2018b, a, 2016, 2015b, a, 2014, 2013). The data presented in this work are available at https://doi.org/10.18160/gcp-2021 (Friedlingstein et al., 2021).