Metal manufacturing is responsible for 8% of global CO2 emissions and if carbon neutrality is to be achieved by 2050, we critically need to transition to more sustainable processes. In this project we address the underlying science and understanding to allow a higher utilisation of low embedded-carbon, higher impurity recycled metal as a feedstock for metal manufacturing. Current manufacturing approaches are highly dependent on energy-intensive primary metal as they rely on tightly controlled compositions with very low impurity contents to provide the required materials properties. We believe that the new understanding needed to provide transformative and efficient methods to manufacture high grade metal alloys using a much higher fraction of lower embedded-carbon recycled material as a feedstock can be delivered by leveraging the combined power of multi-modal X-ray imaging and in-line artificial intelligence. We will develop a new wholistic characterisation system comprising both newly developed hardware and AI algorithms named Artificial Intelligence X-ray Imaging (AIXI) as an intelligent tool to investigate the solidification of impurity-rich alloys in experimental conditions comparable to those found in industrial processes such as continuous casting, direct chill casting, shape casting and additive manufacturing for a wide range of aluminium and steel alloy compositions. AIXI will provide a significant advantage over existing approaches as AI will be embedded in the data acquisition system and used to interpret raw data in real-time, drastically reducing the complexity and time required for data analysis and significantly increasing the analytical power of the system. The new knowledge will allow us to finally understand the role that impurities and minor alloy additions play in the developing solidification microstructure, and to develop methodologies to mitigate their deleterious effects. It will also promote a shift to a more holistic approach for alloy design in which the solidification microstructure is engineered to both provide enhanced properties and to facilitate subsequent downstream processes with minimised environmental impact. The newly acquired knowledge will foster the development of science for `sustainable' alloys, which will: enhance metal recyclability by reducing the need for dilution of recycled scrap with energy intensive primary metal; encourage greater use of lower-grade scrap, widely available in the UK but currently exported; decrease the number of downstream processing steps (process intensification), especially heat treatment practices; simplify component recoverability by reducing the reliance on tight compositions specifications; and enhance materials properties by improving control over the final microstructure. We will uncover and apply the missing science to control phase transformations to create more benign and impurity tolerant microstructures and allow more efficient use of expensive and potentially scarce alloy additions, which will substantially cut resource use in the CO2-intensive metal industries. Furthermore, we envisage that the application of the developed hardware/AI analysis could potentially facilitate rapid scientific development in many fields of materials science and beyond where efficient, rapid collection and analysis of complex and large multi-modal datasets is critical to unlock the necessary understanding

This project aims to compare the energy used in traditional foundry processes and a novel single shot foundry technology, CRIMSON, and to develop a model of the processes that encapsulates the energy content at each stage. This model can then be used to persuade casting designers to use more energy-efficient processes which consider casting quality as well as design flexibility. The UK retains a globally recognised casting expertise, in copper, aluminium and new light-metal alloys that underpins many competitive, technology-based industries vital to keep the UK's aerospace and automotive base ahead of the competition. These industries draw on advanced R&D work carried out by Birmingham's high-profile Casting Research Group.The University of Birmingham has been at the leading edge of casting R&D for many years. Today, it is internationally acknowledged as a front runner, and the CRIMSON technique - Constrained Rapid Induction Melting Single Shot method - is one such technology which is helping the casting industry make a step-change in product quality, manufacturing responsiveness and energy use.A typical light-metal foundry will tend to work in the following way: from 100 kg to several tonnes of metal is melted in a first furnace, held at about 700 oC in a second, transferred into a ladle and finally poured into the casting mould. It can take a shift (8 hours) to use all the melt in a typical batch and any leftover unused melt is poured off to be used again, or becomes scrap. Quality issues also arise, which must be mitigated: during the time for which the melt is held at temperature, atmospheric water is reduced to hydrogen and oxygen. The hydrogen is highly soluble in the metal at this temperature, but as the casting cools and solidifies, the gas is ejected into bubbles. The bubbles become porosity in the solid casting and have a detrimental effect on performance, therefore, as much gas must be removed as possible from the melt. The oxygen forms a thin layer of oxide on the melt surface, which is then inevitably entrained in the liquid metal when it is transferred between the different furnaces and when the metal is finally poured. The oxide layer (or bi-film) is now an inclusion which, again, has a detrimental effect on the material properties. The longer the metal is held liquid, the more hydrogen is absorbed and the thicker the oxide becomes on the surface.At each stage of the process there are energy losses due to oxidation and furnace inefficiencies, casting yields and eventually scrap. So from an initial theoretical 1.1 GJ/tonne required tomelt aluminium it is possible to estimate that each tonne of aluminium castings shipped will actually use about 182 GJ/tonne.Instead of going through this batch process, the CRIMSON method uses a high-powered furnace to melt just enough metal to fill a single mould, in one go, in a closed crucible. It transfers the crucible into an up-casting station for highly computer-controlled filling of the mould, against gravity, for an optimum filling and solidification regime. The CRIMSON method therefore only holds the liquid aluminium for a minimum of time thus drastically reducing the energy losses attributed to hold the metal at temperature. With the rapid melting times achieved, of the order of minutes, there isn't a long time at temperature for hydrogen to be absorbed or for thick layers of oxide to form. The metal is never allowed to fall under gravity and therefore any oxide formed is not entrained within the liquid. Thus higher quality castings are produced, leading to a reduction in scrap rate and therefore reduced overall energy losses.The first challenge in the project is to measure accurately the energy used at each stage in each of the processes investigated and to calculate the energy losses from oxidation and scrap. The second challenge is to incorporate this information into a model that can be used by casting designers and foundry engineers.

This project aims to compare the energy used in traditional foundry processes and a novel single shot foundry technology, CRIMSON, and to develop a model of the processes that encapsulates the energy content at each stage. This model can then be used to persuade casting designers to use more energy-efficient processes which consider casting quality as well as design flexibility. The UK retains a globally recognised casting expertise, in copper, aluminium and new light-metal alloys that underpins many competitive, technology-based industries vital to keep the UK's aerospace and automotive base ahead of the competition. These industries draw on advanced R&D work carried out by Birmingham's high-profile Casting Research Group.The University of Birmingham has been at the leading edge of casting R&D for many years. Today, it is internationally acknowledged as a front runner, and the CRIMSON technique - Constrained Rapid Induction Melting Single Shot method - is one such technology which is helping the casting industry make a step-change in product quality, manufacturing responsiveness and energy use.A typical light-metal foundry will tend to work in the following way: from 100 kg to several tonnes of metal is melted in a first furnace, held at about 700 oC in a second, transferred into a ladle and finally poured into the casting mould. It can take a shift (8 hours) to use all the melt in a typical batch and any leftover unused melt is poured off to be used again, or becomes scrap. Quality issues also arise, which must be mitigated: during the time for which the melt is held at temperature, atmospheric water is reduced to hydrogen and oxygen. The hydrogen is highly soluble in the metal at this temperature, but as the casting cools and solidifies, the gas is ejected into bubbles. The bubbles become porosity in the solid casting and have a detrimental effect on performance, therefore, as much gas must be removed as possible from the melt. The oxygen forms a thin layer of oxide on the melt surface, which is then inevitably entrained in the liquid metal when it is transferred between the different furnaces and when the metal is finally poured. The oxide layer (or bi-film) is now an inclusion which, again, has a detrimental effect on the material properties. The longer the metal is held liquid, the more hydrogen is absorbed and the thicker the oxide becomes on the surface.At each stage of the process there are energy losses due to oxidation and furnace inefficiencies, casting yields and eventually scrap. So from an initial theoretical 1.1 GJ/tonne required tomelt aluminium it is possible to estimate that each tonne of aluminium castings shipped will actually use about 182 GJ/tonne.Instead of going through this batch process, the CRIMSON method uses a high-powered furnace to melt just enough metal to fill a single mould, in one go, in a closed crucible. It transfers the crucible into an up-casting station for highly computer-controlled filling of the mould, against gravity, for an optimum filling and solidification regime. The CRIMSON method therefore only holds the liquid aluminium for a minimum of time thus drastically reducing the energy losses attributed to hold the metal at temperature. With the rapid melting times achieved, of the order of minutes, there isn't a long time at temperature for hydrogen to be absorbed or for thick layers of oxide to form. The metal is never allowed to fall under gravity and therefore any oxide formed is not entrained within the liquid. Thus higher quality castings are produced, leading to a reduction in scrap rate and therefore reduced overall energy losses.The first challenge in the project is to measure accurately the energy used at each stage in each of the processes investigated and to calculate the energy losses from oxidation and scrap. The second challenge is to incorporate this information into a model that can be used by casting designers and foundry engineers.

Natural resources are the foundation of our life on Earth, without which neither our economy nor society can function. However, due to continued resource overconsumption and the rapidly increasing world population, the global demand for natural resources and the related intense pressure on our environment have reached an unprecedented and unsustainable level. A shocking fact is that our cumulative consumption of natural resources over the last 60 years is greater than that over the whole of previous human history. With an anticipated world population of 9.3bn in 2050, the predicted global natural resource consumption will be almost tripled. This level of overconsumption is obviously not sustainable, and there is a compelling need for us to use our advanced science and technology to work with, rather than to exploit, nature. Metallic materials are the backbone of manufacturing and the fuel for economic growth. However, metal extraction and refining is extremely energy intensive and causes a huge negative impact on our environment. The world currently produces 50MT of Al and 2bnT of steel each year, accounting for 7-8% of the world's total energy consumption and 8% of the total global CO2 emission. Clearly, we cannot continue this increasing and dissipative use of our limited natural resources. However, the good news is that metals are in principle infinitely recyclable and that their recycling requires only a small fraction of the energy required for primary metal production. Between 1908 and 2007 we produced 833MT of aluminium, 506MT of copper and 33bnT of steels. It is estimated that more than 50% of this metal still exists as accessible stock in our society. Such metal stock will become our energy "bank" and a rich resource for meeting our future needs. The UK metal casting industry adds £2.6bn/yr to the UK economy, employs 30,000 people, produces 1.14bnT of metal castings per year and underpins the competitive position of every sector of UK manufacturing. However, the industry faces severe challenges, including "hollowing-out" over the past 30 years, increasing energy and materials costs, tightening environmental regulations and a short supply of skilled people. We are now establishing the Future Liquid Metal Engineering Hub to address these challenges. The core Hub activities will be based at Brunel strongly supported by the complementary expertise of our academic spokes at Oxford, Leeds, Manchester and Imperial College and with over £40M investment from our industrial partners. The Hub's long-term vision is full metal circulation, in which the global demand for metallic materials is met by a full circulation of secondary metals (with only limited addition of primary metals each year) through reduced usage, reuse, remanufacture, closed-loop recycling and effective recovery and refining of secondary metals. This represents a paradigm shift for metallurgical science, manufacturing technology and the industrial landscape. The Hub aims to lay down a solid foundation for full metal circulation, demonstrated initially with light metals and then extended to other metals in the longer term. We have identified closed-loop recycling of metallic materials as the greatest challenge and opportunity facing global manufacturing industry, and from this we have co-created with our industrial partners the Hub's research programme. We will conduct fundamental research to deliver a nucleation centred solidification science to underpin closed-loop recycling; we will carry out applied research to develop recycling-friendly high performance metallic materials and sustainable metal processing technologies to enable closed-loop recycling; we will operate a comprehensive outreach programme to engage potential stakeholders to ensure the widest possible impact of our research; we will embed a centre for doctoral training in liquid metal engineering to train future leaders to deliver long-lasting benefits of closed-loop recycling.

The UK metal casting industry is a key player in the global market. It adds 2.6bn/year to the UK economy, employs directly around 30,000 people and produces 1.14 billion tons of metal castings, of which 37% is for direct export (Source: CMF, UK). It underpins the competitive position of every sector of UK manufacturing across automotive, aerospace, defence, energy and general engineering. However, its 500 companies are mainly SMEs, who are often not in a position to undertake the highest quality R&D necessary for them to remain competitive in global markets. The current EPSRC IMRC portfolio does not cover this important research area nor does it address this clear, compelling business need. We propose to establish IMRC-LiME, a 3-way centre of excellence for solidification research, to fill this distinctive and clear gap in the IMRC portfolio. IMRC-LiME will build on the strong metal casting centres already established at Brunel, Oxford and Birmingham Universities and their internationally leading capabilities and expertise to undertake both fundamental and applied solidification research in close collaborations with key industrial partners across the supply chain. It will support and provide opportunities for the UK metal casting industry and its customers to move up the value chain and to improve their business competitiveness. The main research theme of IMRC-LiME is liquid metal engineering, which is defined as the treatment of liquid metals by either chemical or physical means for the purpose of enhancing heterogeneous nucleation through manipulation of the chemical and physical nature of both endogenous (naturally occurring) and exogenous (externally added) nucleating particles prior to solidification processing. A prime aim of liquid metal engineering is to produce solidified metallic materials with fine and uniform microstructure, uniform composition, minimised casting defects and hence enhanced engineering performance. Our fundamental (platform) research theme will be centred on understanding the nucleation process and developing generic techniques for nucleation control; our user-led research theme will be focused on improving casting quality through liquid metal engineering prior to various casting processes. The initial focus will be mainly on light metals with expansion in the long term to a wide range of structural metals and alloys, to eventually include aluminium, magnesium, titanium, nickel, steel and copper. In the long-term IMRC-LiME will deliver: 1) A nucleation-centred solidification science, that represents a fundamental move away from the traditional growth-focused science of solidification. 2) A portfolio of innovative solidification processing technologies, that are capable of providing high performance metallic materials with little need for solid state deformation processing, representing a paradigm shift from the current solid state deformation based materials processing to a solidification centred materials engineering. 3) An optimised metallurgical industry, in which the demand for metallic materials can be met by an efficient circulation of existing metallic materials through innovative technologies for reuse, remanufacture, direct recycling and chemical conversion with limited additions of primary metal to sustain the circulation loop. This will lead to a substantial conservation of natural resources, a reduction of energy consumption and CO2 emissions while meeting the demand for metallic materials for economic growth and wealth creation.